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Ultrasonic vibration can be used for the micromolding of metallic glasses (MGs) due to stress-softening and fast surface-diffusion effects. However, the structural rearrangement under ultrasonic vibration and its impact on the mechanical response of metallic glasses remain a puzzle. In this work, the plastic flow of the Zr 35 Ti 30 Cu 8.25 Be 26.75 metallic glass with the applied ultrasonic-vibration energy of 140 J was investigated by nanoindentation. Both Kelvin and Maxwell-Voigt models have been adopted to analyze the structural evolution during the creep deformation. The increase of the characteristic relaxation time and the peak intensity of relaxation spectra can be found in the sample after ultrasonic vibration. It effectively improves the activation energy of atomic diffusion during the glass transition (E g ) and the growth of the crystal nucleus (E p ). A more homogenous plastic deformation with a weak loading-rate sensitivity of stress exponent is observed in the ultrasonic-vibrated sample, which coincides with the low pile-up and penetration depth as shown in the cross profile of indents. The structural rearrangement under resonance actuation demonstrated in this work might help us better understand the defect-activation mechanism for the plastic flow of amorphous systems.

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