The advanced molybdenum-based rare process experiment (AMoRE) aims to search for neutrinoless double beta decay ($$0\nu \beta \beta $$0νββ) of $$^{100}$$100Mo with $$\sim 100\,\hbox {kg}$$∼100kg of $$^{100}$$100Mo-enriched molybdenum embedded in cryogenic detectors with a dual heat and light readout. At the current, pilot stage of the AMoRE project we employ six calcium molybdate crystals with a total mass of 1.9 kg, produced from $$^{48}$$48Ca-depleted calcium and $$^{100}$$100Mo-enriched molybdenum ($$^{48{{\text {depl}}}}\hbox {Ca}^{100}\hbox {MoO}_{4}$$48deplCa100MoO4). The simultaneous detection of heat (phonon) and scintillation (photon) signals is realized with high resolution metallic magnetic calorimeter sensors that operate at milli-Kelvin temperatures. This stage of the project is carried out in the Yangyang underground laboratory at a depth of 700 m. We report first results from the AMoRE-Pilot $$0\nu \beta \beta $$0νββ search with a 111 kg day live exposure of $$^{48{{\text {depl}}}}\hbox {Ca}^{100}\hbox {MoO}_{4}$$48deplCa100MoO4 crystals. No evidence for $$0\nu \beta \beta $$0νββ decay of $$^{100}$$100Mo is found, and a upper limit is set for the half-life of $$0\nu \beta \beta $$0νββ of $$^{100}$$100Mo of $$T^{0\nu }_{1/2} > 9.5\times 10^{22}~\hbox {years}$$T1/20ν>9.5×1022years at 90% C.L. This limit corresponds to an effective Majorana neutrino mass limit in the range $$\langle m_{\beta \beta }\rangle \le (1.2-2.1)\,\hbox {eV}$$⟨mββ⟩≤(1.2-2.1)eV.
A single crystal scintillation material (Gd0.5–Y0.5)3Al2Ga3O12 (GYAGG) doped with Ce and codoped with Mg at a small concentration was grown by the Czochralski technique and studied for its scintillation properties for the first time.
Calcium molybdate is considered as a very promising scintillator material for experimental studies of rare processes. This paper reports on the production and characterization of a 40 Ca
100MoO 4 scintillator. Using the Czochralski technique, a crystal of high optical quality with total mass 0.55 kg, 42 mm diameter (minimum) and 53 mm 1ength of the cylindrical section was produced from isotopically enriched raw materials, containing 96.1% of 100 Mo and 99.964% of 40 Ca. To satisfy the requirement of low intrinsic radioactivity the purity of the materials was monitored at different stages of the production process and it is shown that the concentration of 238 U and 232 Th in the final crystal does not exceed 0.05 ppb. The scintillation properties of 40 Ca 100 MoO 4 were measured over the 8 -300 K temperature range and it is found that the light yield of the 40 Ca
100MoO 4 crystal is very similar to that of the CaMoO 4 reference scintillator.
This report presents results on the significant improvement of GAGG:Ce based scintillation detector performance with temperature decrease. When temperature of a PMT based detector is lowered to-45 o C, its amplitude response at registration of γ-quanta is improved by 30%; FHHM was found to be better up to factor of 0.85, whereas scintillation kinetics become even faster in crystals co-doped with magnesium and magnesium and titanium. All this opens an opportunity for a wide application of GAGG scintillation detectors, particularly in a combination with SiPM photo-sensors, which signal-to-noise ratio would also improve with temperature decrease.
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