This paper presents the results of the experimental studies of InAs quantum dot overgrowth by a low-temperature GaAs layer at different arsenic vapor pressures. It is revealed that a threefold decrease in the arsenic pressure at a fixed deposition rate of the capping layer leads to a change in the shape of the photoluminescence spectrum of quantum dots with one maximum at the level of 1.19 eV to the shape of the spectrum with two low-energy contributions at the levels of 1.08 and 1.15 eV. Based on the analysis of the power dependences of the photoluminescence spectra, it is found that the low-energy contributions of the photoluminescence of quantum dots overgrown at a low arsenic pressure correspond to the ground-state emission two groups of quantum dots with different average sizes formed during mass transfer in the “quantum dot – wetting layer – matrix” system.
In this paper, we present the results of studying the influence of arsenic pressure in the range of ultra-low values (10^-7-10^-6 Pa) on the processes of modification of In/GaAs(001) droplets with various initial sizes obtained by droplet epitaxy. We experimentally demonstrate that exposure of droplets to the ultralow arsenic flux makes it possible to reduce the droplet size to subcritical sizes while maintaining the initially specified surface density. The exposure of droplet nanostructures in the arsenic flux can be accompanied only by a decrease in their size, which is more typical for droplets obtained at large amounts of indium deposited material. For droplets with a smaller initial size, the formation of rings along the perimeter of the initial droplets and holes inside the rings is typical along with the droplet reduction. We also reveal that the dependence of the relative volume of droplets subjected to diffusion decay in the arsenic flux becomes more significant with a decrease in their initial size.
In this paper, we present a study of the effect of the silicon substrate modification by focused ion beams on subsequent growth of GaAs layers by molecular beam epitaxy. We demonstrate that when samples exposed to the ion irradiation at various accelerating voltages and ion beam passes are annealed in the absence of the arsenic flux, an increase in the depth of the modified Si substrate areas occurs. At the same time, crystallization of gallium accumulations during annealing in the arsenic flux leads to the filling of holes formed during the ion bombardment. We reveal that the growth of GaAs on substrates with areas modified at an accelerating voltage of 30 kV and subjected to subsequent annealing in the arsenic flux at a temperature of 600 °C is accompanied by the formation of nanowires, the density of which increases within areas with a large number of ion beam passes. The results of the conducted research can be used for the development of technological approaches to the formation of GaAs epitaxial layers on Si substrates.
This paper presents the results of experimental studies of the effect of the Ga ion dose during ion-beam treatment of the Si(111) surface using the focused ion beam technique on the GaAs nanowires epitaxial growth processes. A significant difference is revealed between the parameters of nanowire arrays formed on modified and unmodified areas of the Si substrate in this way. It is shown that changing the Ga ions dose from 0.052 to 10.4 pC/μm^2 during ion-beam treatment makes it possible to form GaAs nanowires arrays with a different set of parameters in a single technological cycle with a high degree of localization. The regularities of the influence of the dose of Ga ions during surface modification on the key characteristics of GaAs nanowires (density, diameter, length, and orientation with respect to the substrate surface) are experimentally established.
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