The contact network of granular materials is often divided into strong and weak subnetworks, which play different roles in micromechanics. Within the strong contact network, there exists the largest connected component, that is, the largest cluster, which may connect system boundaries and could be the most important structure in force transmission of the whole system. This paper concerns the particular features of the largest cluster in the strong contact network of granular materials, by considering the combining effects of loading path and particle shape. A series of true triaxial tests with various intermediate principal stress ratios are conducted for granular assemblies of different shaped particles using the discrete element method (DEM). Both the macroscopic stress–strain responses and the microscopic topological changes of the contact network are investigated. It is found that both particle shape and loading path will influence the shear strength and the topological features of the strong network. The threshold (the ratio to the average force) is used to distinguish the strong and weak networks, and a critical threshold can be identified by comparing the network‐based metrics. The largest cluster within the strong network approaching the critical threshold can span the boundaries in each direction with minimum contacts, which occupies a small portion of particles and contacts but transmits a considerable portion of the applied stress. In addition, the similar contribution weight of the largest cluster to the deviatoric stress is identified for granular materials with different particle shapes.