The Plum Rains process is a complex process, and its spatiotemporal variations and influencing factors on different time scales still need further study. Based on a dataset on the Plum Rains in the Yangtze River Delta, from 33 meteorological stations during the period of 1960 to 2012, we investigated the spatiotemporal variations of Plum Rains and their relation with the East Asian Summer Monsoon (EASM), the El Niño-Southern Oscillation (ENSO), and the Pacific Decadal Oscillation (PDO) using an integrated approach that combines ensemble empirical mode decomposition (EEMD), empirical orthogonal function (EOF), and correlation analysis. The main conclusions were as follows: (1) the plum rainfall (i.e., the rainfall during the period of Plum Rains) showed a trend of increasing first and then decreasing, and it had a three-year and six-year cycle on the inter-annual scale and a 13-year and 33-year cycle on the inter-decadal scale. The effect of the onset and termination of Plum Rains and the daily intensity of plum rainfall on plum rainfall on the inter-annual scale was greater than the inter-decadal scale, (2) the EOF analysis of plum rainfall revealed a dominant basin-wide in-phase pattern (EOF1) and a north-south out-of-phase pattern (EOF2), and (3) ENSO and EASM were the main influencing factors in the three-year and six-year periods, respectively.