In the second alloy category, seventeen alloy compositions were prepared, using different additions of Zr, Sc, Ti-B, Sr, Ag, and Si These alloys were further divided into four groups, namely, the Zr-Ti, Zr-Sr, Zr-Sc, and Si alloy groups. Tensile test bars (cooling rate 7°C/s) prepared from these alloys were solutionized for 8h at 490°C then age-hardened at temperatures of 180°C and 220°C for aging times of 2, 4, 6, 10,16, 24, and 48h, and 0.5,1, 1.5, 2, 4, 6, 10, 16, 24, and 48h, respectively. It was observed that combined additions of Zr-Ti Zr-Sr, or Zr-Sc refined the grain size of the base alloy considerably, from 219 um to 104-46 urn, since these elements form primary trialuminide intermetallics including Al3(Sci-x Zr x ), Al3(Sci-x -yZr x Tiy), and AlaZr which act as nucleation sites for o-Al grains, thereby producing fine non-dendritic structures. The refined non-dendritic morphology produced by the combined additions of Zr-Ti Zr-Sr, or Zr-Sc caused a reduction of about 65% in the amount of the AliCu phase in the base alloy, and a reduction in porosity of about 50%. The addition of 2 wt% Si also produced the same reduction levels in the amount of AfeCu and porosity, brought about by the increase in the Al-Si eutectic content. Age-hardening peaks were observed after aging for lOh and 24h at 180°C, and after aging for Ih and 2h at 220°C. The Zr-Sr and Zr-Ti alloy groups displayed the highest level of improvement in the tensile properties of the Al-2wt%Cu base alloy followed by the Zr-Sc and Si alloy groups, in that order. The 0.02wt%Sr-0.7wt%Zr containing alloy produced the highest ultimate tensile and yield strength values of 383 MPa and 326 MPa, respectively, after 4h of aging at 180°C. The strength of the base alloy increased in the Zr-Ti alloy group with an increase in Zr content from 0.15wt% to 0.7wt% after aging at 180°C for lOh. This increase may be variously attributed to Al$Zr and Al3(Zri. x Ti x ) dispersoids acting as heterogeneous nucleation sites for age-hardening phases; to the modifying action of Zr on the S' (AfeCuMg) phase; and to the action of Zr-Ti in producing a refined non-dendritic grain structure. Combined additions of Zr-Sr and Sr-Ti displayed the best elongation levels of all the alloys investigated, as witnessed by the 0.02wt%Sr-0.15wt%Ti-containing alloy and, 0.02wt%Sr-0.7wt%Zr-containing alloy. These improved levels may be the result of the modifying effects of Sr on o-Fe particles, as well as of the roles of Zr and Ti in producing a fine non-dendritic os-Al structure. The 0.02wt%Sr-0.15wt%Ti-containing alloy displayed the highest resistance to softening during aging at 220°C because of the respective modifying and refining effects of Sr and Ti on the microstructure.