specialized to respond to various physical stimuli (e.g., temperature, pressure, and stretching), humans can rapidly and accurately locate and identify objects via haptic perception. [5][6][7] To emulate human skin with haptic pressure sensation, tactile sensors capable of measuring contact pressure/force have been extensively exploited with diverse nanomaterials and nanostructures over the past decade. [8][9][10][11][12][13] For example, Gong et al. proposed a flexible and highly sensitive pressure sensor by sandwiching ultrathin gold nanowire between elastomer sheets that allowed real-time monitoring of arterial blood pressure through skin surface contact. [10] Cao et al. demonstrated enhanced tactile sensitivity for surface texture discerning based on an optimized micropyramid structure assembled with a single-walled carbon nanotube. [13] The general principle of such sensors is to transduce the mechanical stimuli into electrical signals through the effects of piezoelectricity, capacitance, or piezoresistance. [14,15] Tactile sensors made of piezoelectric elements have shown advantages such as high sensitivity, low power consumption, and high response frequency, which make them, especially promising for dynamic pressure measurements such as slip and vibration detection in robotics. [15][16][17] However, the piezoelectric effects are generally temperature-dependent, and not suitable for static pressure measurement due to charge leakage. [18,19] Capacitive sensors can monitor both static and dynamic pressure with the merits of temperature independence and long-term stability but suffer from parasitic effects, complex circuits, and limited working range. [20][21][22] By comparison, piezoresistive sensors have been more predominantly used for tactile sensing due to their simple structure, easy readout, and broad sensing range. [23,24] However, they typically exhibit undesirable hysteresis and signal drift, inducing practical difficulties in high-precision measurements. [18] Besides, other issues such as electromagnetic interference (EMI) susceptibility, electrical safety, and biocompatibility of the electronic components in medical settings, are also common concerns of all aforementioned approaches that impair their widespread applications. [25,26] Recently, there have also been efforts in developing tactile sensors by using ion conductors and ionic luminophores that can convert mechanical stimuli into luminescence. [27,28] These sensors provide visual-tactile feedback with spatially-resolved capability, but suffer from long response