High-damping alloys are finding more and more applications as a passive damping measure in mechanical structures in attempts to eliminate noise and vibration, especially in circumstances where traditional structural damping or system damping methods are not suitable, for example, in high-temperature environments.[1] High-damping alloys have the ability to damp out noise and vibration, and are expected also to possess adequate mechanical properties such as rigidity and strength. In high-temperature working environments, both high damping capacity and strength at elevated temperatures are required. The damping capacity of high-damping alloys (equivalent to the internal friction of a material) is defined as the capacity of a material to convert its mechanical energy of vibration into heat, which is dissipated in the material. With the exception of thermoelastic damping, the majority of damping mechanisms are associated with the stress-induced movement of crystalline defects. Point defects give rise to damping in the range of low to intermediate levels, dislocations give rise to damping levels in the intermediate to high range, and planar defects (twin boundaries and magnetic domain boundaries) give rise to damping levels in the high range.[2] Three groups of high-damping alloys have been developed in the past 50 years, which apply the mechanisms of dislocation damping, ferromagnetic damping, and twinboundary damping, respectively. However, there are some deficiencies in the damping behavior of the alloys, which have affected the application of high-damping alloys. In the case of dislocation-type damping alloys, rearrangement of the pinning points during continued vibration leads to a damping capacity that varies with service time. [2] Similarly, for twin boundarytype damping alloys, it is reported that degradation of damping capacity occurs when they are held at room temperature, which is induced by the diffusion of interstitial carbon atoms to the twin boundaries.[3] And for ferromagnetic high-damping alloys, the damping capacity will be considerably reduced in the presence of a magnetic field or a static load. While the optimization of the damping microstructure is an important research topic for the already developed high-damping alloys, [4][5][6] it is noted that both dislocation damping and boundary damping are influenced by the interstitial impurities in the alloys. While interstitial impurities are easily introduced into the alloys in the conventional fabrication processes, no work has been done to show the advantage of interstitial solid solution atoms in improving the damping capacity of those alloys. We took up the challenge of obtaining a high damping capacity in alloys by making use of the interstitial solid solution atoms. Point defects in crystalline solids can generate a time-dependent strain under the application of an external stress due to the reorientation of the point defects. This phenomenon was experimentally investigated in body-centered cubic (bcc) metals with interstitial impurities of carbo...