“…Conventionally employed electronic materials with pristine forms (e.g., thin-film metals or semiconductors) exhibit a significant increase in electrical resistance with accumulating strain owing to their structural irreversibility. A variety of approaches have been explored to convert intrinsically brittle electronic materials to stress-resilient forms by rationally engineering their physical configurations and dimensions. − Among them, forming the materials into “kirigami” patterns inspired by the ancient paper-cutting art , offers distinguishable advantages for efficiently relieving external stress. − This kirigami patterning employs rows of designed cuts to a planar material, which improves its mechanical stretchability by converting applied tensile stress to torsional stress at specific points between the cuts. − In addition to structural “engineering” approaches, substantive efforts have been used to identify a new form of electronic materials which intrinsically possess suitable crystallinity to enable superior mechanical tolerance. In this endeavor, recently explored two-dimensional (2D) transition-metal dichalcogenides (TMDs) present highly unique and promising aspects. , For instance, they exhibit significantly larger in-plane strain limits over covalently bonded three-dimensional crystals owing to their van der Waals molecular bonding, offering opportunities for futuristic stretchable electronics. , Despite the projected advantages, combining these two different compelling approaches (i.e., converting 2D TMDs into kirigami forms) has been rarely attempted, leaving their anticipated mechanoelectrical superiority largely unexplored.…”