Greenhouse gases (GHGs) in the Earth's atmosphere, including CO 2 , CH 4 , H 2 O, and O 3 , absorb as well as emit infrared radiation. At lower altitudes where the air is dense, they are optically thick to outgoing infrared radiation and thus produce a heating effect. In contrast, at higher altitudes where the air is increasingly tenuous, they become optically thin to outgoing infrared radiation and therefore, produce a cooling effect. Note that the main role of O 3 in the atmosphere is as a solar ultraviolet (UV) absorber in the stratosphere. Therefore, the stratospheric temperature response (and consequently the density response at higher altitudes) to O 3 increases is opposite to that of the other three major GHGs. The stratospheric O 3 trend is not monotonic (Figure 1), and until recently was negative, thus contributing to cooling like the other three GHGs, but for a different reason. Observational and modeling studies found that since the 1960s, the long-term changes of these GHGs have caused warming in the troposphere (∼0.