Understanding the role of spin-orbit coupling (SOC) has been crucial to controlling magnetic anisotropy in magnetic multilayer films [1][2][3][4]. It has been shown that electronic structure can be altered via interface SOC by varying the superlattice structure, resulting in spontaneous magnetization perpendicular or parallel to the plane [5,6]. In lieu of magnetic thin films, we study the similarly anisotropic helimagnet Cr 1/3 NbS2, where the spin polarization direction, controlled by the applied magnetic field, can modify the electronic structure. As a result, the direction of spin polarization can modulate the density of states, and in turn affect the in-plane electrical conductivity. In Cr 1/3 NbS2, we found an enhancement of in-plane conductivity when the spin polarization is out-of-plane, as compared to in-plane spin polarization. This is consistent with the increase of density of states near the Fermi energy at the same spin configuration, found from first principles calculations. We also observe unusual field dependence of the Hall signal in the same temperature range. This is unlikely to originate from the non-collinear spin texture, but rather further indicates strong dependence of electronic structure on spin orientation relative to the plane.
PACS numbers:Despite the fact that its typical energy scale in 3d ferromagnetic metals is small compared to other relevant scales such as band widths, SOC mixes the nature of the spin and orbital components of the Bloch state in a nontrivial way and leads to a variety of electrical transport phenomena e.g. the anomalous Hall effect (AHE), anisotropic magnetoresistance (AMR), and the planar Hall effect. In addition, the recent work in non-collinear magnetically ordered states and the related topological Hall effect [7][8][9] not only has renewed the pivotal role of SOC through the Dzyaloshinskii-Moriya (DM) interaction [10][11][12], but also has presented a possibility to employ these findings for functional components in magnetic devices [13,14]. Non-collinear magnetic ordering is also suggested to possibly manifest spin-orbit coupling in a complex manner, through the DM interaction [12,15,16]. Consequently, the modification of electronic structure by spin-orbit coupling is expected to make in-plane electrical transport sensitive to the magnetization orientation relative to the plane.Cr 1/3 NbS 2 has a layered crystalline structure, in which 3d transition metal Cr atoms are intercalated in the hexagonal 2H-type NbS 2 matrix as trivalent ions and magnetically order at T C = 133 K. The ferromagnetic layers of Cr 3+ lie coplanar with the crystallographic abplanes and the magnetic helix propagates along the caxis with a long pitch of 48 nm, corresponding to 40 unit cells [17]. Its helimagnetic ordering is attributed to the DM interaction, which originates from a broken inversion symmetry shared by all members of space group P 6 3 22 [17][18][19].