Background: At the forefront of the nuclear science, production of new neutron-rich isotopes is continuously pursued at accelerator laboratories all over the world. To explore the currently-unknown territories in the nuclear chart far away from the stability, reliable theoretical predictions are inevitable.Purpose: To provide a reliable prediction of production cross sections taking into account secondary deexcitation processes, both particle evaporation and fission, a new method called TDHF+GEMINI is proposed, which combines the microscopic time-dependent Hartree-Fock (TDHF) theory with a sophisticated statistical compoundnucleus deexcitation model, GEMINI++.Methods: Low-energy heavy ion reactions are described based on three-dimensional Skyrme-TDHF calculations. Using particle-number projection method, production probabilities, total angular momenta, and excitation energies of primary reaction products are extracted from the TDHF wavefunction after collision. Production cross sections for secondary reaction products are evaluated employing GEMINI++. Results are compared with available experimental data and widely-used GRAZING calculations.
Results:The method is applied to describe cross sections for multinucleon transfer processes in MeV) reactions at energies close to the Coulomb barrier. It is shown that the inclusion of secondary deexcitation processes, which are dominated by neutron evaporation in the present systems, substantially improves agreement with the experimental data. The magnitude of the evaporation effects is very similar to the one observed in GRAZING calculations. TDHF+GEMINI provides better description of the absolute value of the cross sections for channels involving transfer of more than one protons, compared to the GRAZING results. However, there remain discrepancies between the measurements and the calculated cross sections, indicating a limit of the theoretical framework that works with a single mean-field potential. Possible causes of the discrepancies are discussed.
Conclusions:In order to perfectly reproduce experimental cross sections for multinucleon transfer processes, one should go beyond the standard self-consistent mean-field description. Nevertheless, the proposed method will provide valuable information to optimize production mechanisms of new neutron-rich nuclei through its microscopic, non-empirical predictions.