1978
DOI: 10.1063/1.437057
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Application of generalized cumulant expansions to the theory of electron spin echo phase memory decay in liquids

Abstract: A generalized cumulant expansion theory for electron spin relaxation in liquids is presented which describes the phase memory decay found in pulse experiments. It is found that for pulse times τ≫τc, the two-pulse electron spin echo envelope decays exponentially, and for motionally narrowed systems, the phase memory decay rate is given by the elements of the Redfield relaxation matrix. For radicals undergoing slow rotational reorientation, the phase memory time is shown to be sensitive to both the rotational co… Show more

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Cited by 4 publications
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“…He had worked as a graduate student with Bob Schwartz on theoretical aspects of electron spin echoes (ESE) in liquids (38). I had succeeded in getting some funds from the NSF to initiate construction of a spin-echo bridge.…”
Section: Time Domain Esr Theory and Methodsmentioning
confidence: 99%
“…He had worked as a graduate student with Bob Schwartz on theoretical aspects of electron spin echoes (ESE) in liquids (38). I had succeeded in getting some funds from the NSF to initiate construction of a spin-echo bridge.…”
Section: Time Domain Esr Theory and Methodsmentioning
confidence: 99%