“…In recent years, nano‐scale reinforcements have become essential to enhance the fiber–matrix interface. [ 15 ] The reinforcements such as carbon nanotube (CNT), [ 16,17 ] SiO 2 , [ 18 ] nanoclay, [ 19,20 ] graphene, [ 21–23 ] CaCO 3 , [ 24 ] and Al 2 O 3 [ 25 ] represented enhancements on the mechanical, thermal and chemical properties of composite materials. On the other hand, halloysite nanotubes (HNTs) are abundant nano particles with tubular 1D structure, large aspect ratio, natural existence, prosperous functionality, good biocompatibility, and high mechanical properties.…”