“…Over the last decade, there has been increased use of data assimilation techniques to constrain model forecasts and reanalyses of atmospheric constituents (e.g., Arellano Jr. et al, 2007;Edwards et al, 2009;Claeyman et al, 2011;Lahoz et al, 2012;Pagowski and Grell, 2012;Bowman, 2013;Gaubert et al, 2014;Hache et al, 2014;Saide et al, 2014;Zoogman et al, 2014;Barré et al, 2015;Bousserez et al, 2016;Mizzi et al, 2016). Assimilation of chemicals can be extended to optimize model inputs such as emissions, thereby providing insight into how to improve the processes that govern the model performance (e.g., Elbern et al, 2007;Barbu et al, 2009;Chatterjee et al, 2012;Miyazaki et al, 2012b;Koohkan et al, 2013;Yumimoto, 2013;Cui et al, 2015;Guerrette and Henze, 2015;Turner et al, 2015).…”