Aerosols modify the Earth's radiative budget through scattering and absorption of solar (shortwave) and terrestrial (longwave) radiation and have large variability in their physical and chemical properties, horizontal and vertical distributions, and feedbacks from other components of the climate system, particularly clouds (Persad & Caldeira, 2018;Ramanathan, 2001). Overall, aerosol climatic effects lead to one of the largest uncertainties in future climate projections (Hinds, 1999;Stocker, 2014). Unlike the effect of well-mixed greenhouse gases, the aerosol radiative effect is stronger at the surface than at the top of the atmosphere (Ramanathan, 2001), with aerosols reducing incoming shortwave radiation through scattering and absorption and increasing incoming longwave radiation through re-emission of the absorbed energy (Chakraborty