Carboxylic acid-functionalized cadmium sulfide/graphitic carbon nitride composite photocatalyst with well-combined interface for sulfamethazine degradation

Cao, Shihai; Jiao, Zhongyi; Chen, Huan; Jiang, Fang; Wang, Xin

doi:10.1016/j.jphotochem.2018.05.030

Cited by 23 publications

(3 citation statements)

References 55 publications

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“…Pathway 2 was chiefly the separation of sulfonyl groups. SMZ lost a sulfonyl group and the C-N bond broke to form P5 and P7 [ 45 ]. Pathway 3 commonly includes the scission of S-N bonds.…”

Section: Resultsmentioning

confidence: 99%

Effects of Sulfamethazine and Cupric Ion on Treatment of Anaerobically Digested Swine Wastewater with Growing Duckweed

Yang

2022

IJERPH

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Duckweed (Spirodela polyrrhiza) has the potential to treat anaerobically digested swine wastewater (ADSW), but the effects of antibiotics and heavy metals in ADSW on the treatment performance and mechanism of Spirodela polyrrhiza are not clear. Herein, an experiment was conducted to investigate the effects of sulfamethazine (SMZ) and cupric ion on NH4+-N and total phosphorus (TP) removal from synthetic ADSW. The activity of superoxide dismutase (SOD) and the contents of photosynthetic pigments, vitamin E, and proteins in duckweed were also evaluated. Under the stress of SMZ, duckweed showed excellent removal efficiency of nutrients, and the results of SOD activity and photosynthetic pigments content indicated that duckweed had good tolerance to SMZ. Interestingly, a combined application of SMZ and cupric ion would inhibit the nutrient removal by duckweed, but significantly increased the contents of photosynthetic pigments, proteins, and vitamin E. In addition, the consequence indicated that high value-added protein and vitamin E products could be produced and harvested by cultivating duckweed in ADSW. Furthermore, possible degradation pathways of SMZ in the duckweed system were proposed based on the analysis with LC-MS/MS. This research proposed a novel view for using duckweed system to remove nutrients from ADSW and produce value-added products under the stress of SMZ and cupric ion.

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“…Pathway 2 was chiefly the separation of sulfonyl groups. SMZ lost a sulfonyl group and the C-N bond broke to form P5 and P7 [ 45 ]. Pathway 3 commonly includes the scission of S-N bonds.…”

Section: Resultsmentioning

confidence: 99%

Effects of Sulfamethazine and Cupric Ion on Treatment of Anaerobically Digested Swine Wastewater with Growing Duckweed

Yang

2022

IJERPH

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“…Moreover, the outstanding development of a combination interface between carboxylic acid-functionalized CdS and g-C 3 N 4 enhanced both stability and separation of photogenerated charge carriers. [47] Table 1. Summary of recently reported functionalized g-C 3 N 4 .…”

Section: Chemical Grafting and Functionalization Of Surface Moietymentioning

confidence: 99%

Surface Physicochemistry Modification and Structural Nanoarchitectures of g‐C₃N₄ for Wastewater Remediation and Solar Fuel Generation

Hasnan

Mohamed

Hir

2021

Adv Materials Technologies

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“…Among different carbon allotropies, graphitic carbon nitride (g-C3N4) has been attracted lots of attention owing to optoelectrical and chemical properties [32][33][34]. Chen et al [35] reported the carboxylic acid -functionalized CdS/g-C3N4 heterojunction as an efficient photocatalyst for sulfamethazine decomposition. The CdS/spherical g-C3N4 photocatalyst was prepared by Wu and Wang et al [36] using the solvothermal method, which showed 93.2 % tetracycline degradation.…”

Section: Introductionmentioning

confidence: 99%

Achieving the Enhanced Photocatalytic Degradation of Ceftriaxone Sodium Using CdS-g-C3N4 Nanocomposite under Visible Light Irradiation: RSM Modeling and Optimization

Attarikhasraghi

Zare

Mehrizad

et al. 2021

J Inorg Organomet Polym

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In this research, the cadmium sulfide -graphite carbon nitride (CdS-g-C3N4) nanocomposite was synthesized and characterized by X-ray diffraction (XRD), Field emission scanning electron microscopy (FESEM), energy-dispersive X-ray spectrometer (EDX), and transmission electron microscopy (TEM) techniques. The photocatalytic activity of asprepared nanocomposite was evaluated in the degradation of ceftriaxone sodium (CTX) antibiotic from aqueous solution under visible light irradiation. The influence of the operational variables such as the amount of photocatalyst (g/L), initial CTX concentration (mg/L), pH, and irradiation time (min) on the photodegradation process was investigated and optimized using response surface methodology (RSM) -central composite design (CCD) model. The maximum degradation percentage (92.55 %) was obtained in the optimal condition, including 0.06 g/L of CdS-g-C3N4 photocatalyst, 15 mg/L of CTX, pH= 10.5, and irradiation time = 81 min. The efficient photocatalytic performance of CdS-g-C3N4 nanocomposite is due to the appropriate alignment of energy levels between the CdS and g-C3N4, which synergistically impact the charge separation and the degradation efficiency of CTX. The kinetics of the photocatalytic degradation process was well described by Langmuir-Hinshelwood's pseudo-first-order model (kapp = 0.0336 min -1 ).

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Carboxylic acid-functionalized cadmium sulfide/graphitic carbon nitride composite photocatalyst with well-combined interface for sulfamethazine degradation

Cited by 23 publications

References 55 publications

Effects of Sulfamethazine and Cupric Ion on Treatment of Anaerobically Digested Swine Wastewater with Growing Duckweed

Effects of Sulfamethazine and Cupric Ion on Treatment of Anaerobically Digested Swine Wastewater with Growing Duckweed

Surface Physicochemistry Modification and Structural Nanoarchitectures of g‐C₃N₄ for Wastewater Remediation and Solar Fuel Generation

Achieving the Enhanced Photocatalytic Degradation of Ceftriaxone Sodium Using CdS-g-C3N4 Nanocomposite under Visible Light Irradiation: RSM Modeling and Optimization

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Carboxylic acid-functionalized cadmium sulfide/graphitic carbon nitride composite photocatalyst with well-combined interface for sulfamethazine degradation

Cited by 23 publications

References 55 publications

Effects of Sulfamethazine and Cupric Ion on Treatment of Anaerobically Digested Swine Wastewater with Growing Duckweed

Effects of Sulfamethazine and Cupric Ion on Treatment of Anaerobically Digested Swine Wastewater with Growing Duckweed

Surface Physicochemistry Modification and Structural Nanoarchitectures of g‐C3N4 for Wastewater Remediation and Solar Fuel Generation

Achieving the Enhanced Photocatalytic Degradation of Ceftriaxone Sodium Using CdS-g-C3N4 Nanocomposite under Visible Light Irradiation: RSM Modeling and Optimization

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Surface Physicochemistry Modification and Structural Nanoarchitectures of g‐C₃N₄ for Wastewater Remediation and Solar Fuel Generation