Abstract:We describe carrier–carrier interaction in self-assembled In0.5Ga0.5As quantum dots (QDs) at room temperature. The spectral shift and linewidth broadening of ground state emission as a function of the excitation density are investigated through near-field single quantum dot photoluminescence spectroscopy. From the viewpoint of excitation density dependent spectral broadening of the ground state emission, we discuss the dephasing process in QDs due to Coulomb interaction.
“…In Refs. [20] and [21] PL spectroscopy measurements revealed homogeneous linewidths of several meV at room temperature. Comparable results have also been found by four-wave mixing experiments [15].…”
Section: Introductionmentioning
confidence: 99%
“…1(a) of Ref. [21] optical spectra are displayed for different excitation intensities. Although a direct comparison of the excitation dependence is not possible, due to uncertainties in the carrier densities generated in those experiments, the general features of the spectra are identical.…”
A microscopic theory is used to study the optical properties of semiconductor quantum dots. The dephasing of a coherent excitation and line-shifts of the interband transitions due to carriercarrier Coulomb interaction and carrier-phonon interaction are determined from a quantum kinetic treatment of correlation processes. We investigate the density dependence of both mechanisms and clarify the importance of various dephasing channels involving the localized and delocalized states of the system.
“…In Refs. [20] and [21] PL spectroscopy measurements revealed homogeneous linewidths of several meV at room temperature. Comparable results have also been found by four-wave mixing experiments [15].…”
Section: Introductionmentioning
confidence: 99%
“…1(a) of Ref. [21] optical spectra are displayed for different excitation intensities. Although a direct comparison of the excitation dependence is not possible, due to uncertainties in the carrier densities generated in those experiments, the general features of the spectra are identical.…”
A microscopic theory is used to study the optical properties of semiconductor quantum dots. The dephasing of a coherent excitation and line-shifts of the interband transitions due to carriercarrier Coulomb interaction and carrier-phonon interaction are determined from a quantum kinetic treatment of correlation processes. We investigate the density dependence of both mechanisms and clarify the importance of various dephasing channels involving the localized and delocalized states of the system.
“…Heitz et al observed a similar behavior for the InAs/GaAs QDs [25], was related to the band-gap shrinkage of the dot and/or barriers due to the Coulomb interaction between carriers [25,26] band-gap renormalisation (BGR). The peak of the PL signal observed for energies below…”
, et al.. Power density and temperature effects on the photoluminescence spectra of InAlAs/GaAlAs quantum dots. Superlattices and Microstructures, Elsevier, 2017, 104, pp.321-330. <10.1016/j.spmi.2017.02.043>. M A N U S C R I P T A C C E P T E D
“…While this approach provides thorough calculation of free-carrier effects, it has been noted that finding the exact parameters which will simulate experimental results remains difficult to produce a match. [10][11][12] Another model developed,…”
We simulate the shape of the density of states (DoS) of the quantum dot (QD) ensemble based upon size information provided by high angle annular dark field scanning transmission electron microscopy (HAADF STEM). We discuss how the capability to determined the QD DoS from micro-structural data allows a MonteCarlo model to be developed to accurately describe the QD gain and spontaneous emission spectra. The QD DoS shape is then studied, with recommendations made via the effect of removing, and enhancing this size inhomogeneity on various QD based devices is explored.
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