The emergence of various data-intensive applications like artificial intelligence, machine learning etc., has highlighted the energy and throughput bottlenecks inherent in existing computing systems. Memory storage is a major component for such data intensive computational platforms. Consequently, memory-centric research investigations to improve the overall energy-efficiency and throughput of a given computing chip is being actively pursued. Exploration of novel memory technologies for high-density on-chip memories and in-memory computing are the key examples of such memory-centric approaches. In this paper, we propose a novel memory-centric scheme based on CMOS SRAM. Our proposal aims at dynamically increasing the on-chip memory storage capacity of SRAM arrays on-demand. The proposed scheme called -Augmented Memory Computing allows an SRAM cell to operate in two different modes 1) the Normal mode and 2) the Augmented mode. In the Normal mode of operation, the SRAM cell functions like a standard 6 transistor (6T) SRAM cell, storing one bit of data in static format. While in the Augmented mode, each SRAM cell can store >1 bit of data (in a dynamic fashion). Specifically, we propose two novel SRAM cells -an 8 transistor (8T) dual bit storage augmented cell and a 7 transistor (7T) ternary bit storage augmented cell. The proposed 8T dual bit SRAM cell when operated in the Augmented mode, can store a static bit of data while also, simultaneously, storing another bit in a dynamic form. Thus, when operated in Augmented mode, the 8T SRAM cell can store two bits of dataone SRAM-like data and one DRAM-like data, thereby increasing or augmenting the memory storage capacity. On the other hand, the proposed 7T ternary bit storage augmented cell can either store a single SRAM data in Normal mode or can be configured to operate in Augmented mode, wherein it can store ternary data (3 levels (0,0), (0,1), (1,0)) in a dynamic manner. Thus, based on the mode of operation, the proposed augmented memory bitcells can either store one static bit of data or >1 bit of data in a dynamic format. We show the feasibility of our proposed bit-cells through extensive simulations at Globalfoundries 22nm FDX node. It is worth mentioning, the novel scheme of augmented memory bit-cells can be seamlessly combined with existing inmemory computing approaches for added energy and throughput benefits.