The formation of
soot in a swirling flow is investigated experimentally
and numerically in the context of biogas combustion using a CO
2
-diluted methane/oxygen flame. Visualization of the swirling
flow field and characterization of the burner geometry is obtained
through PIV measurements. The soot particle size distributions under
different fuel concentrations and swirling conditions are measured,
revealing an overall reduction of soot concentration and smaller particle
sizes with increasing swirling intensities and leaner flames. An axisymmetric
two-dimensional CFD model, including a detailed combustion reaction
mechanism and soot formation submodel, was implemented using a commercial
computational fluid dynamics (CFD) code (Ansys Fluent). The results
are compared with the experiments, with similar trends observed for
the soot size distribution under fuel-lean conditions. However, the
model is not accurate enough to capture soot formation in fuel-rich
combustion cases. In general, soot particle sizes from the model are
much smaller than those observed in the experiments, with possible
reasons being the inappropriate modeling in Fluent of governing mechanisms
for soot agglomeration, growth, and oxidation for CH
4
-CO
2
mixtures.