computing. This requires on-chip integrated photonic devices to have the performances of small volume, low power consumption, and easy integration with other nanophotonic devices. [3,4] As an essential component of on-chip integrated photonic devices, polarization router can separate and steer light with different polarizations of transverse electric (TE) and transverse magnetic (TM) modes into different output ports, so as to realize polarization division multiplex of channels. In the past few years, polarization routers are generally realized based on gratings, [5][6][7][8] optical waveguides, [9][10][11][12] photonic crystals, [13][14][15][16] plasmonic structures, [17][18][19][20] metamaterials [21][22][23] or some other structures. [24][25][26][27] Polarization routers based on gratings or waveguides usually possess simple configurations and high extinction ratio, but the large size restricts the practical applications for onchip dense integration. [5,[7][8][9][10] The routers based on photonic crystals possess high transmittance, but the bandwidth is narrow and the crosstalk is relatively large. [13,16] The plasmonic polarization routers are broadband and have smaller size, but usually possess large loss. [17,18] Polarization routers based on metamaterials have high efficiency, but the fabrication process is complicated and the size is relatively large. [21,23] Large size and low-efficiency excitation of traditional design cause the polarization routers to be difficult to meet the requirements of high-density on-chip integration. Therefore, it is a great challenge Nanophotonic polarization routers, which can separate and steer light with different polarizations of transverse electric and transverse magnetic modes into different output ports, are an essential component of on-chip integrated photonic circuits. By developing an intelligent algorithm that combines the genetic algorithm and the finite element method, various polarization routers possessing different operation bands, different structures, and different materials, which can be easily fabricated and integrated, are successfully designed. On-chip ultrasmall silicon-based polarization routers are experimentally demonstrated in the near-infrared range. The footprint is only 970 nm × 1240 nm, which is the smallest demonstrated. The measured normalized transmission is up to 85% in the near infrared range. Additionally, a broadband highly efficient photon coupler is also achieved based on disordered-grating configurations designed by the intelligent algorithm. This breaks the restrictions of traditional structures, provides a universal platform for the realization of nanophotonic polarization routers, and paves a way for the design and high-density on-chip integration of nanophotonic devices.The ORCID identification number(s) for the author(s) of this article can be found under https://doi.org/10.1002/adom.201902018.With the development of big data age, the requirements for large information capacity is becoming higher and higher. On-chip integrated phot...