“…Fallout and ozone are only of limited use for this purpose as the stratospheric fallout reserves are dependent upon a very irregular and arbitrary "supply", and ozone, in the lower troposphere, is subject to processes of decay varying with time. Measurements from the earth's surface are not subject to these difficulties and have likewise been already conducted at many locations [15,21,26,27,1,14,24,2,46]. This procedure has already been in successful use, for some time, in studying the stratospheric-tropospheric exchange, atmospheric mixing, and problems of global propagation (see for example [28,16,32,49,17,25,24,53,2,46] and others).…”