We observe quantum beats with periodic revivals due to non-linear spacing of Zeeman levels in the ground state of potassium atoms and demonstrate their synchronous optical pumping by double modulation of the pumping light at the Larmor frequency and the revival frequency. We show that synchronous pumping increases the degree of spin polarization by a factor of 4. As a practical example, we explore the application of this double-modulation technique to atomic magnetometers operating in the geomagnetic field range and find that it can increase the sensitivity and reduce magnetic field orientation-dependent measurement errors endemic to alkali-metal magnetometers.PACS numbers: 07.55. Ge, 42.50.Md, 32.30.Dx, 32.80.Bx Periodic revival of quantum beats is a general phenomenon that occurs in multi-level systems with nonlinear energy level spacing [1,2] and has been observed in diverse systems, from one-atom masers [3] and Rydberg states in atoms [4] to molecular vibrational [5] and rotational [6] states. Recently molecular rotational revivals attracted significant attention because of the possibility of using them for alignment of molecules with ultrashort laser pulses [7,8,9,10]. It has been proposed that periodic laser pulses could be used to increase the degree of molecular alignment and maintain it indefinitely [11,12,13,14]. An increase of molecular alignment using two pulses has been demonstrated in [15].Here we show experimentally that appropriately synchronized train of laser pulses can increase in the degree of spin orientation and maintain it indefinitely by synchronously pumping quantum revivals in the groundstate Zeeman levels of an alkali-metal atom. Periodic revivals of quantum beats in Zeeman levels of alkalimetal atoms occur naturally due to non-linear Breit-Rabi mixing [16] and have been modeled in [17]. We observe quantum revivals in K atoms and demonstrate their synchronous pumping by double modulation of the pump laser at both the Larmor and the revival frequencies. We find that it creates a coherently oscillating superposition state with a spin polarization a factor of 4 higher than can be obtained without double modulation for the same average laser power. We also model the effects in other alkali atoms and find that the amount of polarization enhancement increases for systems with a larger number of quantum states.Because the revivals occur in geomagnetic field range of about 0.5 G, our experiments are also directly applicable to optically-pumped alkali-metal magnetometers, which are used in many applications, from archaeology [18] and mineral exploration [19] to searches for a CPviolating electric dipole moment [20]. As was recently discussed in [21,22], Breit-Rabi mixing of Zeeman levels decreases magnetometer sensitivity by splitting the Zeeman resonance into many separate lines. We show that synchronous pumping of quantum revivals largely recovers the signal loss. In addition, we demonstrate that it generates a symmetric resonance lineshape, reducing a systematic effect endemic to most alk...