2020
DOI: 10.1007/s40820-020-0413-7
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Comprehensive Insight into the Mechanism, Material Selection and Performance Evaluation of Supercapatteries

Abstract: HIGHLIGHTS• This article reviewed the recent progress on material challenges, charge storage mechanism, and electrochemical performance evaluation of supercapatteries.• Supercapatteries bridge the gap between supercapacitors (low energy density) and batteries (low power density). Fig. 1 a Ragone plot of various electrochemical energy conversion and storage devices [43]. b Schematic illustration of charge storage mechanism of EDL capacitor in porous carbon electrode. c Representation of EDLC structures: Helmhol… Show more

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Cited by 226 publications
(125 citation statements)
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References 256 publications
(407 reference statements)
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“…SCs are energy storage devices known for high power density, cyclic stability, and environment safety. [ 131 ] In particular, FSCs are potential candidates for high‐performance wearable electronic devices as traditional planar SCs could not meet the lightweight, compactness, flexibility, portability, etc., requirements. An FSC comprises a cathode, an anode and an electrolyte, exactly as conventional SC.…”
Section: Fiber‐shaped Energy Storage Devicesmentioning
confidence: 99%
“…SCs are energy storage devices known for high power density, cyclic stability, and environment safety. [ 131 ] In particular, FSCs are potential candidates for high‐performance wearable electronic devices as traditional planar SCs could not meet the lightweight, compactness, flexibility, portability, etc., requirements. An FSC comprises a cathode, an anode and an electrolyte, exactly as conventional SC.…”
Section: Fiber‐shaped Energy Storage Devicesmentioning
confidence: 99%
“…Gouy and Chapman model further introduced the concept of the diffused layer due to the movement of electrolytic ions which could not hold true for higher concentrations of electrolyte and high charge of electrodes. Later Stern model was presented for a betterdetailed explanation of EDLCs combining Gouy-Chapman model and Helmholtz model (Balasubramaniam et al, 2020;Varghese et al, 2011;Wang, Xu, et al, 2020). EDLC briefly stores charge through bi-layers of polarized ions across the surface of the electrode.…”
Section: Capacitive and Non-capacitive Energy Storagementioning
confidence: 99%
“…Other allotropes of carbon such as graphene, carbon nanotube and composites are available in the development of future supercapacitors. 9,10 Key investigations from this study include: Formulation of colloidal electrolyte recipes containing activated carbon particles, Methodologies and processes of EPD to make practical energy storage electrodes, Impact of electrode calendaring on cell performance, Electrochemical coin cell cycling activities, and Scaling-up EPD studies for pouch cell manufacture and their electrochemical testing activities.…”
Section: Introductionmentioning
confidence: 99%