2023
DOI: 10.1016/j.jcou.2023.102431
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Continuous carbon dioxide electroreduction to formate coupled with the single-pass glycerol oxidation to high value-added products

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Cited by 14 publications
(22 citation statements)
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“…In terms of FE toward HCOO − , a value of 41% was obtained, which is also similar to that obtained in the absence of Bi 2 O 3 particles (39%) and that obtained when the OER is used as the anodic reaction (45%), Figure 3. Under these high current density conditions, similar cell voltages were found in the absence (−6.94 V) 41 and in the presence (−6.91 V) of Bi 2 O 3 particles in the anolyte (Table S1 of the Supporting Information). Consequently, similar ECs of 936 and 909 kW h•kmol −1 were obtained.…”
Section: Resultssupporting
confidence: 63%
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“…In terms of FE toward HCOO − , a value of 41% was obtained, which is also similar to that obtained in the absence of Bi 2 O 3 particles (39%) and that obtained when the OER is used as the anodic reaction (45%), Figure 3. Under these high current density conditions, similar cell voltages were found in the absence (−6.94 V) 41 and in the presence (−6.91 V) of Bi 2 O 3 particles in the anolyte (Table S1 of the Supporting Information). Consequently, similar ECs of 936 and 909 kW h•kmol −1 were obtained.…”
Section: Resultssupporting
confidence: 63%
“…To properly assess the effects of the presence of the Bi 2 O 3 particles in the anolyte, the results obtained here have been compared with those obtained under the same experimental and operating conditions but in the absence of Bi 2 O 3 particles in the anolyte and reported in some of our previous investigations. 41 Also, previous results obtained in comparable experimental and operating conditions but using the OER at commercial dimensionally stable anodes (DSA/O 2 ) (Ir-MMO (mixed metal oxide) on platinum) as anodic process have been included in this comparative analysis. 70 This comparative analysis is displayed in Figure 3 S1.…”
Section: Resultsmentioning
confidence: 99%
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“…A flow cell consisting of a Bi/C cathode and Pt/C anode has been reported for coupling the CO 2 RR with the GOR. 39 While a high formate concentration of 18 g L À1 was obtained by the cathodic CO 2 RR with over 80% FE at 200 mA cm À2 , a low FE of B20% was delivered for formate by the anodic GOR owing to the severe overoxidation evidenced by the high FE of up to 40% for the carbonate product. Wang et al constructed an F, N co-doped carbon nanosheetsupported Ni single atom cathode and carbon cloth-supported CoSe 2 anode to couple the CO 2 RR with the GOR (Fig.…”
Section: Category IIImentioning
confidence: 99%