“…Over the last several years, a large number of scientific papers focused on trivalent thulium ions (Tm 3+ ) as activators in laser-grade materials have been published, because Tm 3+ , together with Ho 3+ [ 1 ], is an excellent candidate for the development of laser sources emitting in the near- and mid-infrared, from 1.5 to 2.3 µm [ 2 ]. As a matter of fact, the most common bulk matrices (i.e., crystals and transparent polycrystalline ceramics [ 3 ])—such as YAG [ 3 , 4 , 5 , 6 , 7 , 8 , 9 , 10 , 11 ], Lu 2 O 3 [ 12 , 13 , 14 , 15 , 16 ], Sc 2 O 3 [ 17 , 18 , 19 , 20 , 21 ], Y 2 O 3 [ 22 , 23 , 24 , 25 ], YLF [ 26 , 27 ], CaF 2 [ 28 , 29 , 30 ], LuAG [ 31 , 32 , 33 ]—were developed and studied achieving good performance in terms of laser output power, short pulse duration, and broad range of tunability (from 1.84 to 2.07 µm).…”