2018
DOI: 10.1038/s41566-018-0304-3
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Controlling the polarization and vortex charge of attosecond high-harmonic beams via simultaneous spin–orbit momentum conservation

Abstract: Optical interactions are governed by both spin and angular momentum conservation laws, which serve as a tool for controlling light-matter interactions or elucidating electron dynamics and structure of complex systems. Here, we uncover a form of simultaneous spin and orbital angular momentum conservation and show, theoretically and experimentally, that this phenomenon allows for unprecedented control over the divergence and polarization of extreme-ultraviolet vortex beams. High harmonics with spin and orbital a… Show more

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Cited by 173 publications
(99 citation statements)
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References 62 publications
(118 reference statements)
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“…One particularly relevant example is the three-foldsymmetric trefoil field present in the 'bicircular' HHG configurations [22][23][24][25][26][34][35][36][37][38][39][40][41] used to produce circularlypolarized harmonics. This field consists of two counterrotating circularly-polarized drivers at different frequencies, and exhibits the same configuration after a polarization rotation by an angle 2π/n, with n ≥ 3.…”
mentioning
confidence: 99%
“…One particularly relevant example is the three-foldsymmetric trefoil field present in the 'bicircular' HHG configurations [22][23][24][25][26][34][35][36][37][38][39][40][41] used to produce circularlypolarized harmonics. This field consists of two counterrotating circularly-polarized drivers at different frequencies, and exhibits the same configuration after a polarization rotation by an angle 2π/n, with n ≥ 3.…”
mentioning
confidence: 99%
“…XUV/X-ray pulses with OAM are of particular interest for certain classes of experiments 14,15 , preferably in combination with pulse durations in the attosecond regime 16 . To date high-order harmonics in the XUV with OAM have been observed in laser-atom interactions, operating at a moderate intensity () level 1722 . With progress made in FEL beams 23 , producing intense, attosecond, ultrafast XUV pulses with OAM is a challenge that has yet to be met.…”
Section: Introductionmentioning
confidence: 99%
“…The spin angular momentum (SAM) of light also plays an important role in those applications, e.g. to control polarization and OAM in attosecond pulses [6].…”
Section: Introductionmentioning
confidence: 99%