The main goal of our work is the laser fabrication of nanostructured materials including the nanoand microclusters for control of electrical, optical and other properties of obtained structures. First, we took an opportunity to select nanoparticles in various sizes and weights and also in topology distribution for some materials (carbon, Ni, PbTe, etc). Second, for a deposited extended array of nanoparticles we used a method of laser-induced nanoparticle fabrication in colloid and deposition metal (and/or oxide) nanoparticles from colloidal systems (LDPCS) to obtain the multilayered nanostructures with controlled topology, including the fractal cluster structures (for Ni, Pb Te et al). Electrophysical properties are analyzed for such nanocluster systems as well. A brief analogy of the obtained nanocluster structures with a quantum correlated state evidence is carried out.