Gallium
nitride (GaN) film delamination is an important process
during the fabrication of GaN light-emitting diodes (LEDs) and laser
diodes. Here, we utilize 520 nm femtosecond laser pulses, exploiting
nonlinear absorption rather than single-photon absorption such as
in conventional laser lift-off (LLO) employing excimer or Q-switched
laser sources. The focus of this study is to investigate the influence
of laser scanning speed and integrated fluence corresponding to laser
energy per area during the LLO processing of GaN LED chips and their
resulting structural properties. Because both the sapphire substrate
and InGaN/GaN heterostructures are fully transparent to the emission
of the laser system, a key question is related to the impact of laser
pulses on the quality of a thin film structure. Therefore, several
characterization methods (i.e., scanning electron microscopy, atomic
force microscopy, X-ray diffraction, Raman spectroscopy, and electroluminescence
spectroscopy) were employed to understand the material modifications
made by femtosecond LLO (fs-LLO). We demonstrated that by adjusting
the laser scanning speed, smooth GaN surfaces and good crystal quality
could be obtained regardless of the existing delamination of metal
contact, which then slightly downgraded the LED performance. Here,
the integrated fluence level was set in the range of 2.6–4.4
J/cm2 to enable the fs-LLO process. Moreover, two mitigation
strategies were developed and proven to improve the optoelectrical
characteristics of the lifted-off LEDs (i.e., modification of the
processing step related to the metal creation and reduction of laser
energy).