Low radioactive material screening is becoming essential for rare event search experiments, such as neutrinoless double beta decay and dark matter searches in underground laboratories. A gaseous time projection chamber (TPC) can be used for such purposes with large active areas and high efficiency. A gaseous TPC with a Micromegas readout plane of approximately 20×20 cm 2 is successfully constructed for surface alpha contamination measurements. We have characterized the energy resolution, gain stability, and tracking capability with calibration sources. With the unique track-related background suppression cuts of the gaseous TPC, we have established that the alpha background rate of the TPC is 0.13±0.03 µBq/cm 2 , comparable to the leading commercial solutions.