In this study, we
demonstrate sustainable conductive screen printing
ink containing graphite nanoplates (GNPs) prepared by means of combining
shear and ultrasonication exfoliation processes with the aid of mixed-solvent
strategy of isopropanol (IPA)–water mixtures. The screen printed
GNP ink features high conductivity of 4.66 × 104 S/m,
green preparation, low manufacturing cost and has the potential for
industrial scale-up productions. We first benchmark the GNP conductive
ink and screen printed samples to investigate the rheology of the
ink and its compatibility for industrial production. The high loading
GNP ink is further applied to scalable and efficient production of
ultrahigh frequency (UHF) radiofrequency identification (RFID) tag
antenna and reader antenna. A low-cost, accurate wireless liquid sensing
system capable of sensing the content of the liquids via machine learning
data sets by feedforward neural network is demonstrated for ubiquitous
IoT sensing applications. The experimental results demonstrate that
the GNP ink printed RFID tags and reader antennas can provide satisfactory
read range and performance for many practical RFID applications, such
as inventory and security. Furthermore, the printed RFID wireless
sensor incorporating neural network machine learning can accurately
label the content of colorless, transparent, and unidentified liquids,
illustrating the potential in low-cost, green, and industrial scalable
production of GNP conductive ink printed RFID antennas and sensing
systems for massive IoT applications deployment enabling ubiquitous
wireless connectivity.