Ultrabroadband laser sources are highly desirable in a wide variety of modern science disciplines ranging from physics, chemistry and materials science to information communications and processing. Here we present the design and fabrication of a chirped periodically poled lithium niobate (CPPLN) nonlinear photonic crystal that supports multiple orders of quasiphase matching with finite bandwidth and allows for the simultaneous broadband generation of second and third harmonics with high conversion efficiency. Moreover, the chirp rate has a significant influence on the conversion efficiency and bandwidth. The CPPLN scheme offers a promising approach for the construction of short-wavelength laser sources and enables the generation of the three primary colors-red, green and blue-from a single crystal, which may have potential applications in large-screen laser displays. Keywords: chirped periodically poled lithium niobate; quasiphase matching; second-harmonic generation; third-harmonic generation INTRODUCTION Ultrabroadband laser sources are highly desirable in a wide variety of modern science disciplines ranging from physics, chemistry and materials science to information communications and processing. Laser gain media that are capable of short-pulse generation are available but limited, and they cover only a small portion of the optical spectrum. Shortly after the creation of the first laser in 1960, the door to nonlinear optics was opened because of the discovery of second-harmonic generation (SHG).1 Broad-bandwidth and high-conversion-efficiency SHG, third-harmonic generation (THG), higher-order-harmonic generation and various frequency-mixing and parametric-conversion processes have all provided fascinating routes toward the considerable expansion of the spectral range of laser sources.To realize high-efficiency SHG, THG and other optical parametric processes, nonlinear optical materials are required to simultaneously satisfy the phase-matching condition and possess large nonlinear optical coefficients in the phase-matching direction. Although many natural nonlinear crystals have large nonlinear coefficients in certain directions, proper phase matching cannot always be achieved because of the dispersion of the material. Thus, the optical birefringent properties of certain birefringent nonlinear crystals are often utilized to compensate for the material dispersion and achieve phase matching. However, the stringent conditions for birefringent phase matching greatly limit the extension of the optical frequency. As an alternative approach, quasiphase matching (QPM), which was first proposed in 1962, 2 launched a new era in nonlinear optics because of several advantages it offers over conventional birefringence phase matching in the frequency-conversion process. These advantages include phase matching in materials that have high nonlinear optical coefficients but