Groundwater supplies ∼40% of irrigation and household and ∼30% of industrial water use globally (Döll et al., 2012). The generally high-quality water, long residence time, and strong resilience to climate variability (Cuthbert et al., 2019) make groundwater a dependable freshwater resource in many (semi)arid areas, which has led to a rapid increase in groundwater use, especially to sustain rising water demands for increased food production (Pokhrel et al., 2015; Wada et al., 2014). Such groundwater overexploitation has caused an alarming rate of aquifer storage depletion worldwide (Gleeson et al., 2012; Pokhrel et al., 2015; Wada et al., 2010), making groundwater use fundamentally unsustainable that has not only impacted water supplies, but also gravely altered natural hydrologic regimes and deteriorated ecosystem health (Gleeson et al., 2012; Siebert et al., 2010). Hydrologically, groundwater acts as a buffer that directly modulates soil moisture and is coupled to surface water through a relatively slow, two-way water exchange; groundwater converges to streams and lakes as baseflow and recharges naturally by water percolating down from the surface (de