Negative
exchange bias is usually discovered in ferromagnetic (FM)/antiferromagnetic
(AFM) heterostructures after a field-cooling (FC) process. Relatively,
positive exchange bias (PEB) is a rarely observed phenomenon. So far,
almost all of the models for PEB whether undergoing FC or zero-field-cooling
(ZFC) treatment have been explained by an interaction of strong AFM
coupling at the interface. In this work, by selecting a special material
of SrFeO3–x
as the AFM layer, coupled
with FM-La0.7Sr0.3MnO3 (LSMO), we
obtain a novel PEB effect of the bilayer after ZFC measurement, of
which the shift directions are unfixable and dependent on the initial
magnetization direction. Based on a transient magnetic field to control
the remanence (M
r) direction of LSMO at
room temperature and then cooling below the T
N of SrFeO3–x
without any
magnetic field disturbance, the shift direction can be locked only
toward the transient magnetic field. Combined with experimental results
and first-principles calculations, we propose that the above phenomena
are explained as the field-induced AFM phase of SrFeO3–x
transforming into the FM phase at an FM coupling
bilayer interface. Thus, our finding may provide a new approach to
realize and tune the zero-field-cooling PEB with FM coupling heterostructures.