Center for the Evolution of the Elements, USA Background: Dust grains condensed in the outflows of pre-solar classical novae should have been present in the proto-solar nebula. Candidates for such pre-solar nova grains have been found in primitive meteorites and can in principle be identified by their isotopic ratios, but the ratios predicted by state-of-the-art 1D hydrodynamic models are uncertain due to nuclear-physics uncertainties.Purpose: To theoretically calculate the thermonuclear rates and uncertainties of the 34 S(p,γ) 35 Cl and 34g,m Cl(p,γ) 35 Ar reactions and investigate their impacts on the predicted 34 S/ 32 S isotopic ratio for pre-solar nova grains.Method: A shell-model approach in a (0+1)hω model space was used to calculate the properties of resonances in the 34 S(p,γ) 35 Cl and 34g,m Cl(p,γ) 35 Ar reactions and their thermonuclear rates. Uncertainties were estimated using a Monte-Carlo method. The implications of these rates and their uncertainties on sulfur isotopic nova yields were investigated using a post-processing nucleosynthesis code. The rates for transitions from the ground state of 34 Cl as well as from the isomeric first excited state of 34 Cl were explicitly calculated.Results: At energies in the resonance region near the proton-emission threshold many negativeparity states appear. Energies, spectroscopic factors and proton-decay widths are reported. The resulting thermonuclear rates are compared with previous determinations.
Conclusions:The shell-model calculations alone are sufficient to constrain the variation of the 34 S/ 32 S ratios to within about 30%. Uncertainties associated with other reactions must also be considered, but in general we find that the 34 S/ 32 S ratios are not a robust diagnostic to clearly identify presolar grains made from nova ejecta.