2018
DOI: 10.1364/oe.26.006692
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Doppler-free spectroscopy with a terahertz quantum-cascade laser

Abstract: We report on the Doppler-free saturation spectroscopy of a molecular transition at 3.3 THz based on a quantum-cascade laser and an absorption cell in a collinear pump-probe configuration. A Lamb dip with a sub-Doppler linewidth of 170 kHz is observed for a rotational transition of HDO. We found that a certain level of external optical feedback is tolerable as long as the free spectral range of the external cavity is large compared to the width of the absorption line.

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Cited by 26 publications
(13 citation statements)
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“…Despite the very low generated power (generally tens of nW, requiring liquid-He cooled detectors), such a wide-tunability approach has produced, in about fifteen years, plenty (several tens) of significant spectroscopic results (e.g., [6,[18][19][20][21][22][23]). However, after a comparable time-span, THz QCLs have provided mostly proof-of-principle spectroscopic results [10,[24][25][26] to date, thus paying the price for insufficient tunability in regard to spectroscopy.…”
Section: Introductionmentioning
confidence: 99%
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“…Despite the very low generated power (generally tens of nW, requiring liquid-He cooled detectors), such a wide-tunability approach has produced, in about fifteen years, plenty (several tens) of significant spectroscopic results (e.g., [6,[18][19][20][21][22][23]). However, after a comparable time-span, THz QCLs have provided mostly proof-of-principle spectroscopic results [10,[24][25][26] to date, thus paying the price for insufficient tunability in regard to spectroscopy.…”
Section: Introductionmentioning
confidence: 99%
“…The current accuracy (∼10 −9 ) , achieved in a direct-absorption configuration, was limited by the Doppler linewidth of the measured absorption profiles. However, improvement of the order of magnitude is possible by implementing more advanced setups [26,37]. To this purpose, higher THz power levels, in the order of a few µW and not yet available with our source, are desirable.…”
Section: Introductionmentioning
confidence: 99%
“…This further limitation can be overcome using sub-Doppler spectroscopic techniques, that are precluded to DC-FCs-based DCS, but can be implemented in our spectrometer, thanks to the significantly higher output power provided by a QCL-FC. Indeed, saturation effects and pump and probe setups have been implemented with QCLbased spectrometers 59,60 , although no metrological-grade measurements have been obtained yet. Finally, although having low finesse values, newly developed THz resonant cavities 61 Fig.…”
Section: Discussionmentioning
confidence: 99%
“…Full control of FCs, i.e., of linewidth and phase of teeth and spacing between them, as well as of their shape, that means getting control on the overall number and on the intensity pattern of the manifold [51] is the key challenge to widen the application spectrum of FCs. In particular, phase control and a significant increase of the intensity of each tooth (e.g., hundreds µW power range), together with the assessment of a stable FC operation over the entire operational range of the QCL, will make it easier to access the nonlinear interaction regime [52]. Saturation of gas-phase molecular lines is a straightforward example of application that could be accompanied by cavity-enhanced setups, although the cavity finesse reported to date, at THz frequencies, is very limited [53,54].…”
Section: Applications and Perspectivesmentioning
confidence: 99%