USE of nano-sulfur (NS) as a suspension to mitigate calcium carbonate (CaCO 3 ) of calcareous sandy soil is a new strategy and has not yet been tested. In a pot experiment, this study evaluated four NS suspensions containing 15, 30, 60, and 90 kg NS ha −1 , plus the control (distilled water only, 0 NS). Pots were incubated under laboratory conditions for two months. Then, total, active, and active/total CaCO 3 , as well as the CaCO 3 -related properties were estimated. The suspension containing 90 kg NS ha −1 was superior, while that containing 30 kg NS ha −1 was optimum. However, from an economic perspective, the suspension containing 15 kg NS ha −1 was preferred. With the optimum suspension, active, total, and active/total CaCO 3 reduced by about 24%, 40%, and 22% compared to the control, respectively. Furthermore, the CaCO 3 -related properties, such as pH decreased by 0.48 unit and sodium adsorption ( Na-adsorption ) ratio by 18%, while soluble Ca 2+ , K + , SO 4 2− , water stable aggregate index, and macro-to micro-pores ratio increased by about 100%, 44%, 19%, 33%, and 60% compared to the control, respectively. In general, the optimal active CaCO 3 for better soil properties improvement is less than 10%. The NS suspension has a high corrective power on CaCO 3 and its related properties in the short term (60 days). However, regular application is recommended to continue pH reduction and neutralize CaCO 3 . Therefore, NS suspension may be an effective option when an immediate reaction from the amendment is needed, especially at critical stages of growth.