“…In general, this work has shown a strategy to synthesize CsPbBr 3 with an electrochemical substrate (PbO 2 ) that has fewer problems that those of conventional chemical–mechanical methods. Hopefully, it can facilitate relevant research on CsPbBr 3 , a widely applied perovskite due to its own advantages in various fields (solar cells, photodetectors, photocatalysis, lasers, light-emitting diodes, and resistive switching memories). − More importantly, it has shown a high tunability to synthesize perovskites of different contents with different optoelectronic properties, with even wider prospects in different types of applications, such as in two-terminal tandem solar cells, photodetectors in the fields of imaging and optical communication (such as MAPbI 2.55 Br 0.45 ), memories (such as CsPbBrI 2 ), lasers (such as MAPbBr 3 ), etc. − Finally, the versality of the whole method has also been tested for different substrates, especially textured substrates that are often used as the upper antireflex layer in solar cells. , We initially tried to conformally deposit a layer of the perovskite film on a textured crystalline silicon cell by the electrochemical strategy, which illustrates the versatility of the strategy and provides a new idea for the simple preparation of two-terminal perovskite solar cells (as shown in Figure S7).…”