The available power in a flowing fluid is proportional to the cube of its velocity, and this feature indicates the potential for generating substantial electrical energy by exploiting the direct piezoelectric effect. The present work is an experimental investigation of a self-excited piezoelectric energy harvester subjected to a uniform and steady flow. The harvester consists of a cylinder attached to the free end of a cantilevered beam, which is partially covered by piezoelectric patches. Due to fluid–structure interaction phenomena, the cylinder is subjected to oscillatory forces, and the beam is deflected accordingly, causing the piezoelectric elements to strain and thus develop electric charge. The harvester was tested in a wind tunnel and it produced approximately 0.1 mW of non-rectified electrical power at a flow speed of 1.192 m s−1. The aeroelectromechanical efficiency at resonance was calculated to be 0.72%, while the power per device volume was 23.6 mW m−3 and the power per piezoelectric volume was 233 W m−3. Strain measurements were obtained during the tests and were used to predict the voltage output by employing a distributed parameter model. The effect of non-rigid bonding on strain transfer was also investigated. While the rigid bonding assumption caused a significant (>60%) overestimation of the measured power, a non-rigid bonding model gave a better agreement (<10% error).