“…Aiming for this demand, electric voltage control of magnetism by designing ferromagnetic/ferroelectric (FM/FE) heterostructures via non-volatile polarization charge [7][8][9][10] or non-volatile strain derived from the underneath FE layer has been proved to be an efficient method in recent years. The ferroelectric crystals of PbZr 1−x Ti x O 3 (PZT) [16], Pb(Mg 1/3 Nb 2/3 ) 0.7 Ti 0.3 O 3 (PMN-PT) [17], and [Pb(Zn 1/3 Nb 2/3 )O 3 ] x -[PbTiO 3 ] 1−x (PZN-PT) [18] so on, are commonly adapted as a FE layer for their large piezoelectric property, and electric control of magnetization of the adjacent FM layer such as CoFeB [19][20][21][22], FeCo [23], Ni(Fe or Co) [24][25][26], and Co-based Heusler alloys [27][28][29][30][31][32][33][34] have been successfully demonstrated. The converse magnetoelectric (CME) coupling effect in FM/FE heterostructures contains the piezostrain-mediated effect [36][37][38], exchange bias-mediated effect [39,40], and charge-mediated effect [8,9].…”