“…Lithium niobate ( , LN) is one of the most important synthetic crystals and has been dubbed as the “silicon of photonics” for its excellent properties such as relatively high refractive index, wide transparent window, low absorption losses, large nonlinear optical coefficient, outstanding electro-optical response, good temperature stability and others [ 41 , 42 , 43 ]. Particularly, with the progress in thin-film LN on insulator, it has emerged as promising platform for ultracompact photonic devices, such as low-loss waveguides [ 44 , 45 ], high Q resonators [ 46 , 47 , 48 ], metasurfaces [ 49 , 50 ], optical modulators [ 51 , 52 , 53 , 54 , 55 , 56 ], and second harmonic generation [ 57 , 58 , 59 , 60 ]. However, LN’s high hardness and inactive chemical properties make its processing difficult, which severely limits its application in nano-devices and integrated optics.…”