We propose and demonstrate spin manipulation by magnetically controlled modulation of pure spin currents in cobalt/copper lateral spin valves, fabricated on top of the magnetic insulator Y 3 Fe 5 O 12 (YIG). The direction of the YIG magnetization can be controlled by a small magnetic field. We observe a clear modulation of the nonlocal resistance as a function of the orientation of the YIG magnetization with respect to the polarization of the spin current. Such a modulation can only be explained by assuming a finite spin-mixing conductance at the Cu/YIG interface, as it follows from the solution of the spin-diffusion equation Spintronics is a rapidly growing field that aims at using and manipulating not only the charge, but also the spin of the electron, which could lead to faster data processing, nonvolatility, and lower electrical power consumption as compared to conventional electronics [1]. Sophisticated applications such as hard-disk read heads and magnetic random access memory (MRAM) have been introduced in the last two decades.Further progress could be achieved with pure spin currents, which are an essential ingredient in an envisioned spin-only circuit that would integrate logics and memory [2]. The most basic unit in such a concept is the spin analog to the transistor, in which the manipulation of pure spin currents is crucial. The original proposal by Datta and Das [3], which is also applicable to pure spin currents [4], suggested a spin manipulation that would arise from the spin precession due to the spin-orbit interaction modulated by an electric field (Rashba coupling). However, a fundamental limitation appears here, because the best materials for spin transport are those showing the lowest spin-orbit interaction and, therefore, there has been no success in electrically manipulating the spins and propagating them at the same environment, with few exceptions [4].Alternative ways to control pure spin currents are thus desirable. One could take advantage of the spin-mixing conductance concept [5,6] at nonmagnetic metal (NM)/ferromagnetic insulator (FMI) interfaces, which governs the interaction between the spin currents present at the NM and the magnetization of the FMI. This concept is the basis of new spindependent phenomena, including spin pumping [6][7][8][9][10][11][12], spin Seebeck effect [6,13], and spin Hall magnetoresistance (SMR) [6,[14][15][16][17][18]. In these cases, a NM with large spin-orbit coupling is required to convert the involved spin currents into charge currents via the inverse spin Hall effect [19].In this Rapid Communication, we demonstrate an alternative way of modulating pure spin currents based on a magnetic, instead of electric, gating. To that end, we use lateral spin valves (LSVs). These devices allow an electrical injection and detection of pure spin currents in a NM channel by using * f.casanova@nanogune.eu ferromagnetic (FM) electrodes in a nonlocal configuration [20][21][22][23][24][25][26][27][28][29]. The LSVs have been fabricated on top of a FMI, in order to enab...