“…Later, other bichromophoric molecular systems, such as compounds III and IV were studied in solution and in supersonic jets in order to elucidate the mechanisms of intra-EET and intra-ELT. [26][27][28][29][30][31][32][33][34][35][36][37][38][39][40] EET has significant implications in biological systems, [41][42][43] energy transfer dye laser (ETDL) operation, [44][45][46][47][48][49][50] in the realization of molecular electronic devices, [51][52][53] in photodynamic therapy, 54 in light harvesting, 55,56 in photochemical synthesis, 57,58 in developing optical fiber sensors for pH determination in physiological systems, 59 in the determination of the conformation of macromolecules, [60][61][62][63][64] and in the elucidation of the photophysical behavior of large molecules. 65 The purpose of this Review is to discuss progress made in understanding the photophysics and the mechanism of intra-EET within the general framework of radiative and nonradiative processes in molecules.…”