Metallic glasses possess unique properties, such as high strength and high hardness; thus, much attention has been paid to the development of new alloy systems with good mechanical properties. [1][2][3][4] Meanwhile, the mechanical properties of the numerous metallic glasses available have been investigated from different aspects. With the development of the focus-ion-beam (FIB) technique, the size effect on the mechanical properties of metallic glasses on the micrometer scale has also been determined. [5][6][7][8][9][10] These studies found that there is little size effect on the strength, but great effect on the plastic-deformation ability of metallic glasses. [5][6][7][8] Moreover, multiple shear bands were found to be operating in the samples and the plastic strain was in the form of a shear-band burst. [5][6][7][8] In addition, the effect of the geometry on the mechanical response in metallic glasses has also been studied. For example, Lewandowski et al. [11] and Lu et al. [12] investigated the effect of pressure on the yielding and fracture of metallic glasses under tension or compression. In contrast to the catastrophic shear failure in uniaxial compression, the metallic glasses exhibited a large plastic deformation of more than 10% under confinement. [12] In addition, rolling has been applied, to induce profuse shear bands and large deformation and study the evolution of the free volume, [13][14][15] and also to reveal the effect of pre-existing shear bands on the mechanical properties of metallic glasses. [16] Meanwhile, it has been found that the residual stress on the surface of metallic glasses is also useful for improving their mechanical properties. [17] Recently, the mechanical properties of metallic glasses under biaxial tensile loading were studied by the small punch test (SPT). [18][19][20] It was interesting to find that the metallic glasses could be controlled to create regularly arrayed, fine, multiple shear bands under the SPT, indicating that metallic glasses essentially have a good plastic-deformation capability and thus high ductility under suitable loading conditions. The findings showed that the initiation and propagation of shear bands in metallic glasses strongly depend on the stress state. However, under the SPT, some metallic glasses show a faint shear-deformation capability, such as Ti-based metallic glass, which exhibits a significantly unstable shear deformation and a different failure mode to that of Zr-based metallic glass. [20] Therefore, in this communication, the shear-deformation behavior of a Ti-based metallic glass under multiaxial confinement is evaluated and analyzed using the SPT. We confirm that under multiaxial confinement, the sheardeformation capability of a metallic glass can be greatly improved, and that the failure modes can also be changed under this confinement. Figure 1 shows the load-deflection curves of samples S1 and S2, subjected to the SPT. The maximum deflection of sample S1 was 0.63 mm, and the initial stiffness was 2.98 kN mm À1 . However, with confin...