In top-pair events where at least one of the tops decays semileptonically, the identification of the lepton charge allows us to tag not only the top quark charge but also that of the subsequent b quark. In cases where the b also decays semileptonically, the charge of the two leptons can be used to probe CP violation in heavy flavor mixing and decays. This strategy to measure CP violation is independent of those adopted so far in experiments, and can already constrain non standard model sources of CP violation with current and near future LHC data. To demonstrate the potential of this method we construct two CP asymmetries based on same-sign and opposite-sign leptons and estimate their sensitivities. This proposal opens a new window for doing precision measurements of CP violation in b and c quark physics via high p T processes at ATLAS and CMS. Introduction.-The copious production of top quarks at the LHC is usually exploited to explore various top properties or search for new heavy resonances. However, it also opens up the possibility to perform flavor precision measurements. Here we suggest to use the top quark decay products in order to probe CP violation (CPV) in heavy flavor mixing and decays.All existing analyses of CPV in B physics rely on a coherent production of b " b pairs, either from the decay of a b " b resonance or from gluon splitting, where the total b flavor charge at production vanishes. However, top physics gives another source of b's, and due to the large top mass and small width, to a good approximation, a top decay yields a definite nonzero b flavor charge. This charge can be unambiguously tagged at the time of decay by the charge of the lepton daughter of the W (originating from the top). In cases where the b also decays semileptonically, we can construct two CP asymmetries, one in which the latter lepton and the one from the W are of the same sign, and the other with opposite signs. In principle, with a good mass resolution one can also use hadronic decay modes of the b; however, this would be hard to achieve in the near future at ATLAS and CMS.To make our discussion more concrete, let us consider the interesting result obtained by the D0 collaboration at the Tevatron on the CP-violating like-sign dimuon asymmetry [1]: