Diesel particulate matter (DPM) generated as vehicular
exhaust
is one of the main sources of atmospheric soot. These soot particles
have been known to cause adverse health problems in humans and cause
acute environmental problems. Despite great efforts for minimizing
soot production, research on the disposal and recycling of inevitable
diesel soot is scarce. However, DPM consists mainly of carbonaceous
soot (DS) that can be easily utilized as a photothermal material for
solar desalination. Recently, interfacial solar steam generation using
three-dimensional (3D) structures has gained extensive attention.
3D-structured hydrogels have exhibited incredible performance in solar
desalination owing to their tunable physicochemical properties, hydrophilicity,
intrinsic heat localization, and excellent water transport capability.
Herein, a novel DS-incorporated 3D polyvinyl alcohol (PVA)-based hydrogel
is proposed for highly efficient solar desalination. The polymer network
incorporated with purified DS (DSH) achieved an excellent
evaporation rate of 3.01 kg m–2 h–1 under 1 sun illumination due to its vertically aligned water channels,
hydrophilicity, and intrinsic porous structure. In addition, the DSH-PVA hydrogel could generate desalinated water efficiently
(2.5 kg m–2 h–1) with anti-salt
fouling properties. The present results would motivate the utilization
and recycling of waste materials like DS as photothermal materials
for efficient, low-cost, and sustainable solar desalination.