To achieve such excellent electrical properties, thin-film deposition by a high-vacuum system, such as sputtering, have been widely used. [9][10][11] Such processes usually require high cost for device fabrication. In contrast, the use of solution-based materials, especially for metal precursors used in sol-gel chemistry, has attracted significant interest over the past few years. [12][13][14][15][16][17] To achieve a thin-film oxide material based on the solgel method, a high-temperature thermal annealing process is usually necessary. It is necessary to remove the organic ligands and promote the condensation reaction to obtain a metal-oxide (MO) thin film from a xerogel structure. However, high-temperature treatment may limit further applications on flexible or plastic substrates. To date, a few techniques have been reported to overcome these drawbacks. Deep ultraviolet (DUV) or near-infrared (NIR) annealing have already been proposed as the critical step for fabricating thin-film oxide semiconductor devices. Kim et al., [18] Bolat et al., [19] and Moon et al. [20] showed that DUV or NIR annealing at low environmental temperatures can be successfully used to obtain thin-film devices with good carrier mobility and electrical properties. Furthermore, we recently showed that the use of NIR dyes can significantly improve the NIR laser curing of sol-gel indium-zinc-oxide (IZO) materials and allow their use as gas sensors. [21] One of the key parameters for the laser curing of MO precursors is to generate high absorption and efficient conversion to thermal energy. Because the sol-gel layers have an intrinsic low absorption in the NIR, it is necessary to add absorbers in the thin film to generate a local temperature increase. Highly conjugated organic molecules (NIR dyes), carbon black, and carbon nanotubes are potential candidates. Gold nanoparticles (Au NPs) have also proved their utility. Under light excitation, significant thermal effects can be generated, which are known as thermoplasmonic effects. [22][23][24][25][26][27] They correspond to the damping of a plasmon resonance, which creates a temperature increase at the surface of NP that depends on several parameters such as irradiance of the incident light, irradiated area, light wavelength, nature and morphology, surface density, nature of the surrounding medium, and the substrate. [28] In specific conditions, temperature increases such as several hundreds of degrees are achievable and have been used to trigger several Here, a new method is proposed for preparing gold nanoparticles (Au NPs)/ indium-zinc-oxide (IZO) nanocomposite thin films based on photothermal mechanisms with near-Infrared (NIR) laser annealing, which allows integrating the nanomaterial on fragile substrates such as thin glass, plastic sheets, or 3D printed pieces. The Au NPs are first prepared by NIR laser dewetting of a thin Au layer. Then, the Au NPs are used to locally cure the semiconductor material and provide suitable electronic properties owing to their efficient thermoplasmonic effect...