“…However, in our simulation, the tuning effect still exists even in the cases of rigid sliding where the effect of the external field/current on the atomic configuration is eliminated, as shown in Figure S13, indicating that pure electronic behaviors could also affect friction. An electrostatic adhesion/repulsion force induced by the external field is also considered to be the reason for the friction tuning effect in some research. − , This is qualitatively correct according to our calculations: i.e., when the electrostatic force is an adhesive force, the sliding barrier will probably increase, and vice versa, as shown in Figure S14. However, from a quantitative point of view, in our experiment, the increases in adhesion force are less than 2% when the bias voltage is 500 mV, as shown in Figure S15, which cannot fully account for the more than 80% lateral force increase in the fcc region at this bias voltage (Figure e,f).…”