2020
DOI: 10.1039/c9sc04367e
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From wavelike to sub-diffusive motion: exciton dynamics and interaction in squaraine copolymers of varying length

Abstract: We measure excitation energy transport in conjugated polymers using direct observation of exciton pair dynamics.

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Cited by 42 publications
(39 citation statements)
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“…[11][12][13][14] Among the latter squaraines are promising compounds that, due to their strong excitonic interaction with visible light combined with semiconducting properties, [15][16][17] have been widely implemented into photovoltaic light harvesting [18][19][20] and sensing [21][22][23][24] devices and subjected to fundamental molecular excitonic studies. [25][26][27][28][29] Especially appealing are the environmental robustness and the polymorphic structural variety [30,31] that merge into a functional self-patterning of microcrystalline thin films. [32] To eventually allow for in vivo operation of such optoelectronic device, fabrication on a biocompatible substrate is necessary.…”
Section: Introductionmentioning
confidence: 99%
“…[11][12][13][14] Among the latter squaraines are promising compounds that, due to their strong excitonic interaction with visible light combined with semiconducting properties, [15][16][17] have been widely implemented into photovoltaic light harvesting [18][19][20] and sensing [21][22][23][24] devices and subjected to fundamental molecular excitonic studies. [25][26][27][28][29] Especially appealing are the environmental robustness and the polymorphic structural variety [30,31] that merge into a functional self-patterning of microcrystalline thin films. [32] To eventually allow for in vivo operation of such optoelectronic device, fabrication on a biocompatible substrate is necessary.…”
Section: Introductionmentioning
confidence: 99%
“…20 Recently, fifth-order 2Q CMDS has been used to study exciton-exciton interactions in molecular aggregates. 13,[21][22][23][24] Fifth-order 2Q CMDS allows for measurement of both rephasing and non-rephasing 2Q signals 25 and allows for a time delay between pump and probe pulses, which may help to avoid the non-resonant response seen in third-order 2Q spectra.…”
Section: Introductionmentioning
confidence: 99%
“…Fractional differential equations play an important role in different areas of sciences, engineering, and mathematics such as modeling of anomalous diffusive, 1‐4 subdiffusive systems, 5 wave propagation phenomena, 6‐8 soliton dynamics, 9 viscoelasticity, diffusion, 10‐13 plasma physics, 14 and wave phenomena 15‐18 . A fractional diffusion‐wave equation is an integro‐differential equation which is obtained from the classical diffusion or wave equation by replacing the first or second order time derivative term by a fractional derivative of order α with α>0 6 .…”
Section: Introductionmentioning
confidence: 99%