“…Wide band gap semiconductors are commercially used in short-wavelength (blue) light-emitting diodes (LED) and lasers. They are expected to usher applications in high-power, high-speed, and robust optoelectronic devices that can operate in harsh environments . Wide band gap semiconductors are also emerging as attractive materials for integrated photonics, nanophotonics, and nonlinear optoelectronics. − In this context, phosphides and nitrides of gallium (GaP and GaN) are important. , Different nonlinear optical properties of these materials, such as harmonic generation, self-phase modulation, four-wave mixing, and multiphoton absorption, have been extensively investigated. ,,− Among them, multiphoton absorption is relevant for the functionality of photodetectors, lasers, and LEDs.…”